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Its only if you have an additional video card that you enable crossfire.
its already on!! just plug and play!!
If you only have a single 4870x2, there shouldn't even be a crossfire tab in CCC. It's always on unless you disable Catalyst AI in the 3D tab.
You DISABLE crossfire. The reason its not in CCC is becuase you only have one card. The 4870x2 is considered one card.. no crossfire. There is a chip on the card that takes care of this already.
But cross fire is enabled by default for me.